Periodic Oscillations of the Frequency-Dependent Photoelectric Cross Sections of Surface States: Theory and Experiment

Abstract

High-resolution angle-resolved photoemission spectroscopy is employed to study surface states on the Cu(111) surface, with use of synchrotron radiation in the energy range $18<~\hslash \omega <~120$ eV. The results reveal a novel periodic oscillatory behavior in surface-state emission intensity which leads to identification of additional new surface states. A spectral decomposition theory is proposed to explain the physical origin of the oscillations. It describes the measured intensity profiles and predicts that the oscillations are universal for all surface states.