Electron-phonon coupling and electron self-energy in electron-doped graphene: Calculation of angular-resolved photoemission spectra
- 9 November 2007
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 76 (20), 205411
- https://doi.org/10.1103/physrevb.76.205411
Abstract
We obtain analytical expressions for the electron self-energy and the electron-phonon coupling in electron-doped graphene using electron-phonon matrix elements extracted from density functional theory simulations. From the electron self-energies we calculate angle-resolved photoemission spectra (ARPES). We demonstrate that the measured kink at from the Fermi level is actually composed of two features, one at due to the twofold-degenerate mode, and a second one at due to the mode. The electron-phonon coupling extracted from the kink observed in ARPES experiments is roughly a factor of 5.5 larger than the calculated one. This disagreement can be only partially reconciled by the inclusion of resolution effects. Indeed, we show that a finite resolution increases the apparent electron-phonon coupling by underestimating the renormalization of the electron velocity at energies larger than the kink positions. The discrepancy between theory and experiments is thus reduced to a factor of . From the linewidth of the calculated ARPES we obtain the electron relaxation time. A comparison with available experimental data in graphene shows that the electron relaxation time detected in ARPES is almost two orders of magnitudes smaller than that measured by other experimental techniques.
Keywords
This publication has 22 references indexed in Scilit:
- Mind the gapNature Materials, 2007
- Effect of Electron-Electron Interactions on the Conductivity of Clean GraphenePhysical Review Letters, 2007
- Quasiparticle dynamics in grapheneNature Physics, 2006
- First direct observation of Dirac fermions in graphiteNature Physics, 2006
- Minimal conductivity in bilayer grapheneZeitschrift für Physik B Condensed Matter, 2006
- Theoretical Explanation of Superconductivity inPhysical Review Letters, 2005
- Coexistence of sharp quasiparticle dispersions and disorder features in graphitePhysical Review B, 2005
- A review of electron–phonon coupling seen in the high‐Tc superconductors by angle‐resolved photoemission studies (ARPES)Physica Status Solidi (b), 2004
- Kohn Anomalies and Electron-Phonon Interactions in GraphitePhysical Review Letters, 2004
- The Band Theory of GraphitePhysical Review B, 1947