Defective, Porous TiO2 Nanosheets with Pt Decoration as an Efficient Photocatalyst for Ethylene Oxidation Synthesized by a C3N4 Templating Method

Abstract
We report herein a C3N4 templating method for successfully synthesizing defective, porous TiO2 nanosheets with Pt decoration as an efficient photocatalyst for C2H4 oxidation. During the synthetic procedure, C3N4 not only acts as a 2D template to direct synthesize porous TiO2 nanosheets (TiO2-NS) but also facilitates oxygen vacancy formation on TiO2. The resultant TiO2-NS shows enhanced UV and visible light photoactivites toward C2H4 oxidation as compared to blank TiO2 (TiO2-B) prepared without C3N4 template. Subsquently, Pt nanoparticles are homogeneously decorated onto the surface of TiO2-NS. The as-obtained Pt-TiO2-NS exhibits efficient photocatalytic activity and stability toward ethylene oxidation.
Funding Information
  • Ministry of Science and Technology of the People's Republic of China (2013CB933203)
  • Natural Science Foundation of Fujian Province (2014H0054, 2015J0544)
  • National Natural Science Foundation of China (21373224, 21577143)
  • Chinese Academy of Sciences