Evidence for a Ferromagnet—Spin-Glass Transition inPdFeMn

Abstract
Measurements of the low-field ac susceptibility on ternary alloys of Pd + 0.35 at.% Fe and a Mn concentration of 0 to 8 at.% reveal, for three distinct regimes of Mn concentration, (a) a giant-moment ferromagnetism, (b) a high-temperature ferromagnetic phase followed by a lower-temperature spin-glass transition, and (c) a spin-glass phase. Our results for the susceptibility and the Tc phase diagram are satisfactorily explained by the spin-glass theory of Sherrington and Kirkpatrick.