High-Energy Spin Dynamics inLa1.69Sr0.31NiO4

Abstract

To test the prediction that the dispersion of the magnetic resonance in superconducting ${\mathrm{Y}\mathrm{B}\mathrm{a}}_2{\mathrm{C}\mathrm{u}}_3{\mathrm{O}}_{6+x}$ is similar to magnons in an incommensurate antiferromagnet, we have mapped out the spin dynamics in a stripe-ordered nickelate, ${\mathrm{L}\mathrm{a}}_{2-x}{\mathrm{S}\mathrm{r}}_x{\mathrm{N}\mathrm{i}\mathrm{O}}_4$, with $x\simeq 0.31$, using inelastic neutron scattering. We observe spin-wave excitations up to 80 meV emerging from the incommensurate magnetic peaks with a surprisingly large and almost isotropic spin velocity: $\hslash c_s\sim 0.32\mathrm{e}\mathrm{V}\AA$. A comparison indicates that the inferred spin-excitation spectrum is not, by itself, an adequate model for the magnetic resonance feature of the superconductor.