Recent advances and perspectives on light emitting diodes fabricated from halide metal perovskite nanocrystals
- 14 December 2019
- journal article
- review article
- Published by Royal Society of Chemistry (RSC) in Journal of Materials Chemistry C
- Vol. 7 (46), 14412-14440
- https://doi.org/10.1039/c9tc03978c
Abstract
With the growing demand for the next-generation light emitting diode (LED) display and lighting, considerable progress has been realized in the development of various LEDs for research and consumer market. Among diverse emitting materials, all-inorganic perovskite CsPbX3 (X = Cl, Br, I) nanocrystals (NCs) have emerged as active and promising candidates in LEDs due to their high photoluminescence quantum yield (PLQY), high color purity and tunable emission. Over the past four years, a deeper understanding and higher efficiency have been achieved in CsPbX3 NC-based LEDs. These encouraging facts foreshadow the further progress and commercialization in this burgeoning field. Herein, the recent advancements in CsPbX3 NC-based LEDs have been reviewed. The synthesis and passivation methods of CsPbX3 NCs are firstly introduced. Then we summarize the approaches for the fabrication of highly efficient and stable LEDs based on CsPbX3 NCs, including the modification of emitting layers and optimization of structures. Finally, some challenges and possible solutions are suggested for the development of CsPbX3 NC-based LEDs.Funding Information
- National Natural Science Foundation of China (21673150, 21703146, 51802206)
- Natural Science Foundation of Jiangsu Province (BK20180097, BK20180846)
- Higher Education Discipline Innovation Project
- Collaborative Innovation Center of Suzhou Nano Science and Technology
- Priority Academic Program Development of Jiangsu Higher Education Institutions
This publication has 206 references indexed in Scilit:
- Transforming Hybrid Organic Inorganic Perovskites by Rapid Halide ExchangeChemistry of Materials, 2015
- Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color GamutNano Letters, 2015
- Composition-dependent photoluminescence intensity and prolonged recombination lifetime of perovskite CH3NH3PbBr3−xClxfilmsChemical Communications, 2014
- Bright light-emitting diodes based on organometal halide perovskiteNature Nanotechnology, 2014
- Cation-Induced Band-Gap Tuning in Organohalide Perovskites: Interplay of Spin–Orbit Coupling and Octahedra TiltingNano Letters, 2014
- Chloride Inclusion and Hole Transport Material Doping to Improve Methyl Ammonium Lead Bromide Perovskite-Based High Open-Circuit Voltage Solar CellsThe Journal of Physical Chemistry Letters, 2014
- High Open-Circuit Voltage Solar Cells Based on Organic–Inorganic Lead Bromide PerovskiteThe Journal of Physical Chemistry Letters, 2013
- Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic CellsJournal of the American Chemical Society, 2009
- The life and times of the LED — a 100-year historyNature Photonics, 2007
- High intensity photoluminescence of microcrystalline CsPbBr3 films: Evidence for enhanced stimulated emission at room temperatureCurrent Applied Physics, 2005